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A Novel Acrylic Intercalated Hydrotalcite for the Removal of Heavy Metal Ions from Aqueous Solution: Isotherm, Kinetics, Thermodynamics and Mechanism


Paper Type 
 Contributed Paper
Title 
 A Novel Acrylic Intercalated Hydrotalcite for the Removal of Heavy Metal Ions from Aqueous Solution: Isotherm, Kinetics, Thermodynamics and Mechanism
Author 
 Wei Zhao, Youning Chen and Yuhong Li
Email 
 xysyzw@126.com
Abstract:
In this paper, due to the anion exchange between the hydrotalcite layers, the functional nano-acrylic pillared hydrotalcite(AA-LDH) were prepared via back-mixing precipitation method with acrylic acid as the intercalation modifier. AA-LDH was characterized by Fourier transform infrared spectroscopy (FT-IR), X-ray diffraction (XRD) and scanning electron microscopy (SEM). The adsorption performance of AA-LDH for Pb(II), Cu(II), Zn(II) and Cd(II) was investigated. The maximum adsorption capacities of the AA-LDH were up to 4.35 mmol g-1 for Pb(II), 3.67 mmol g-1 for Cu(II), 1.75 mmol g-1 for Zn(II) and 1.23 mmol g-1 for Cd(II) at pH 5.0. The effects of pH on the adsorption suggested that the adsorption of metal ions was governed mainly by the chelation interaction. The adsorption isotherms of the three metal ions were best described by the Langmuir model, and their adsorption kinetics followed the pseudo second-order kinetic equation. The adsorption equilibrium was reached for the four ions within 3h. The adsorption of the three concerned metal ions was hardly affected by common coexisting ions such as Na(I), K(I), Ca(II) and Mg(II), whereas they were slightly decreased when Fe(II) coexisted in the solution, which illustrates the selective adsorption of Pb(II), Cu(II), Zn(II) and Cd(II) from wastewater. The AA-LDH has a good desorption rate and reusability. These findings suggest that the AA-LDH could be potentially applied to the efficient removal of heavy metal ions from waste water.
Start & End Page 
 1055 - 1067
Received Date 
 2019-11-09
Revised Date 
Accepted Date 
 2020-01-03
Full Text 
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Keyword 
 intercalated hydrotalcite, adsorption, heavy metal ion, wastewater, mechanism
Volume 
 Vol.47 No.5 (September 2020)
DOI 
Citation 
 Zhao W., Chen Y. and Li Y., A Novel Acrylic Intercalated Hydrotalcite for the Removal of Heavy Metal Ions from Aqueous Solution: Isotherm, Kinetics, Thermodynamics and Mechanism, Chiang Mai Journal of Science, 2020; 47(5): 1055-1067.
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