Uniaxial Stress Dependence of Dielectric Properties of Poled Ceramics in Lead Magnesium Niobate-Lead Zirconate Titanate System
Supattra Wongsaenmai*, Supon Ananta, Ekarat Meechoowas and Rattikorn Yimnirun* Author for corresponding; e-mail address: spnuy@hotmail.com
Volume: Vol.30 No.2 (AUGUST 2003)
Research Article
DOI:
Received: 9 April 2003, Revised: -, Accepted: 10 May 2003, Published: -
Citation: Wongsaenmai S., Ananta S., Meechoowas E. and Yimnirun R., Uniaxial Stress Dependence of Dielectric Properties of Poled Ceramics in Lead Magnesium Niobate-Lead Zirconate Titanate System, Chiang Mai Journal of Science, 2003; 30(2): 81-93.
Abstract
In this study, effects of uniaxial stress on the dielectric properties of poled ceramics in PMN-PZT system are investigated. The ceramics with a formula (x)Pb(Mg1/3Nb2/3)O3-(1-x)Pb(Zr0.52Ti0.48)O3 or (x)PMN-(1-x)PzT when x = 0.0, 0.1, 0.3, 0.5, 0.7, 0.9 and 1.0 are prepared by a conventional mixed-oxide method. Phase formation behavior and microstructural features of these ceramics are studied by an X-rays diffraction (XRD) and a scanning electron microscopy (SEM) methods, respectively. In addition, other physical properties, e.g, firing shrinkage and density, are measured. The dielectric properties under the uniaxial stress of the poled PMN-PZT ceramics are observed at stress levels up to 5 MPa using a uniaxial compressometer. It is found that with increasing applied stress the dielectric constant of the PZT-rich compositions increases slightly, while that of the PMN-rich compositions decreases. On the other hand, the dielectric loss tangent for most of the compositions first rises and then drops with increasing applied stress.